Stergios Piligkos

Professor

Department of Chemistry
Universitetsparken 5
2100 København Ø
- piligkos@chem.ku.dk
- https://piligkos.kiku.dk
- https://sites.google.com/view/piligkosgroup/home
Phone: +4535320118

ORCID: 0000-0002-4011-6476

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2024
Published
Proof-of-Concept Quantum Simulator Based on Molecular Spin Qudits
Chicco, S., Allodi, G., Chiesa, A., Garlatti, E., Buch, C. D., Santini, P., De Renzi, R., Piligkos, Stergios & Carretta, S., 2024, In: Journal of the American Chemical Society. 146, 1, p. 1053-1061 9 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Structural isomerism-tuned magnetisation relaxation dynamics in lanthanide coordination complexes
Hansen, S. H., Buch, C. D. & Piligkos, Stergios, 2024, ChemRxiv, 11 p.
Research output: Working paper › Preprint
2023
Published
A bis-calix[4]arene-supported [CuII₁₆] cage
Wilson, L. R. B., Coletta, M., Singh, M. K., Teat, S. J., Brookfield, A., Shanmugam, M., Mcinnes, E. J. L., Piligkos, Stergios, Dalgarno, S. J. & Brechin, E. K., 2023, In: Dalton Transactions. 52, 26, p. 8956-8963 8 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Dipolar-Coupled Entangled Molecular 4f Qubits
Bode, B. E., Fusco, E., Nixon, R., Buch, C. D., Weihe, Høgni & Piligkos, Stergios, 2023, In: Journal of the American Chemical Society. 145, 5, p. 2877-2883 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Long aliphatic chain derivatives of trigonal lanthanide complexes
Zhou, Y., Buch, C. D., Hansen, Steen Hansgaard & Piligkos, Stergios, 2023, In: Dalton Transactions. 52, 25, p. 8792-8799 8 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2022
Published
Analysis of vibronic coupling in a 4f molecular magnet with FIRMS
Kragskow, J. G. C., Marbey, J., Buch, C. D., Nehrkorn, J., Ozerov, M., Piligkos, Stergios, Hill, S. & Chilton, N. F., Dec 2022, In: Nature Communications. 13, 1, 10 p., 825.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
High cooperativity coupling to nuclear spins on a circuit quantum electrodynamics architecture
Rollano, V., de Ory, M. C., Buch, C. D., Rubin-Osanz, M., Zueco, D., Sanchez-Azqueta, C., Chiesa, A., Granados, D., Carretta, S., Gomez, A., Piligkos, Stergios & Luis, F., 6 Oct 2022, In: Communications Physics. 5, 1, 9 p., 246.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Spin-Lattice Relaxation Decoherence Suppression in Vanishing Orbital Angular Momentum Qubits
Buch, C. D., Kundu, K., Marbey, J. J., van Tol, J., Weihe, Høgni, Hill, S. & Piligkos, Stergios, 2022, In: Journal of the American Chemical Society. 144, 38, p. 17597–17603 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
The coordination chemistry of p-tert-butylcalix[4]arene with paramagnetic transition and lanthanide metal ions: an Edinburgh Perspective
Wilson, L. R. B., Coletta, M., Evangelisiti, M., Piligkos, Stergios, Dalgarno, S. J. & Brechin, E. K., 2022, In: Journal of the Chemical Society. Dalton Transactions. 51, 11, p. 4213–4226 14 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2021
Published
Magnetic Archimedean Tessellations in Metal–Organic Frameworks
Chen, H., Voigt, L., Kubus, M., Mihrin, D., Mossin, S., Larsen, R. W., Kegnæs, S., Piligkos, Stergios & Pedersen, K. S., 8 Sep 2021, In: Journal of the American Chemical Society. 143, 35, p. 14041-14045 5 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Design of pure heterodinuclear lanthanoid cryptate complexes
Buch, C. D., Hansen, S. H., Mitcov, D., Tram, C. M., Nichol, G. S., Brechin, E. K. & Piligkos, Stergios, 2021, In: Chemical Science. 20, p. 6983–6991 9 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Exploiting host–guest chemistry to manipulate magnetic interactions in metallosupramolecular M₄L₆ tetrahedral cages
Scott, A. J., Vallejo, J., Sarkar, A., Smythe, L., Regincós Martí, E., Nichol, G. S., Klooster, W. T., Coles, S. J., Murrie, M., Rajaraman, G., Piligkos, Stergios, Lusby, P. J. & Brechin, E. K., 2021, In: Chemical Science. 12, 14, p. 5134-5142 9 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
[(V^IVO)₂M^II₅] (M = Ni, Co) Anderson wheels
Fraser, H. W. L., Payne, E. H., Sarkar, A., Wilson, L. R. B., Mitcov, D., Nichol, G. S., Rajaraman, G., Piligkos, Stergios & Brechin, E. K., 2021, In: Dalton Transactions. 50, 36, p. 12495-12501 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
[Cr^III₈Ni^II₆]ⁿ⁺ Heterometallic Coordination Cubes
O’connor, H. M., Sanz, S., Scott, A. J., Pitak, M. B., Klooster, W. T., Coles, S. J., Chilton, N. F., Mcinnes, E. J. L., Lusby, P. J., Weihe, Høgni, Piligkos, Stergios & Brechin, E. K., 2021, In: Molecules. 26, 3, 9 p., 757.
Research output: Contribution to journal › Journal article › Research › peer-review
2020
Published
Functionalized Trigonal Lanthanide Complexes: A New Family of 4f Single-Ion Magnets
Buch, C. D., Hansen, S. H., Tram, C. M., Mitcov, D. & Piligkos, Stergios, 16 Nov 2020, In: Inorganic Chemistry. 59, 22, p. 16328-16340 13 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Hard X-ray magnetochiral dichroism in a paramagnetic molecular 4f complex
Mitcov, D., Platunov, M., Buch, C. D., Reinholdt, A., Døssing, Anders Rørbæk, Wilhelm, F., Rogalev, A. & Piligkos, Stergios, 2020, In: Chemical Science. 11, 31, p. 8306-8311 6 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Lanthanide cryptate monometallic coordination complexes
Buch, C. D., Mitcov, D. & Piligkos, Stergios, 2020, In: Dalton Transactions. 49, 39, p. 13557-13565 9 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2019
Published
Molecular multifunctionality preservation upon surface deposition for a chiral single-molecule magnet
Mitcov, D., Pedersen, A. H., Ceccato, M., Gelardi, R. M., Hassenkam, Tue, Konstantatos, A., Reinholdt, A., Sørensen, M. A., Thulstrup, Peter Waaben, Vinum, M. G., Wilhelm, F., Rogalev, A., Wernsdorfer, W., Brechin, E. K. & Piligkos, Stergios, 1 Jan 2019, In: Chemical Science. 10, 10, p. 3065-3073 9 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Determination of the electronic structure of a dinuclear dysprosium single molecule magnet without symmetry idealization
Perfetti, M., Gysler, M., Rechkemmer-Patalen, Y., Zhang, P., Taştan, H., Fischer, F., Netz, J., Frey, W., Zimmermann, L. W., Schleid, T., Hakl, M., Orlita, M., Ungur, L., Chibotaru, L., Brock-Nannestad, Theis, Piligkos, Stergios & Van Slageren, J., 2019, In: Chemical Science. 10, 7, p. 2101-2110 10 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2018
Published
Chemical tunnel-splitting-engineering in a dysprosium-based molecular nanomagnet
Sørensen, M. A., Hansen, U. B., Perfetti, M., Pedersen, K. S., Bartolome, E., Simeoni, G. G., Mutka, H., Rols, S., Jeong, M., Zivkovic, I., Retuerto Millan, M., Arauzo, A., Bartolome, J., Piligkos, Stergios, Weihe, Høgni, Doerrer, L. H., van Slageren, J., Rønnow, H. M., Lefmann, Kim & Bendix, Jesper, 1 Dec 2018, In: Nature Communications. 9, 9 p., 1292.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
A simple methodology for constructing ferromagnetically coupled Cr(III) compounds
Fraser, H. W. L., Smythe, L., Dey, S., Nichol, G. S., Piligkos, Stergios, Rajaraman, G. & Brechin, E. K., 2018, In: Dalton Transactions. 47, 24, p. 8100-8109 10 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Coherent Manipulation of a Molecular Ln-Based Nuclear Qudit Coupled to an Electron Qubit
Hussain, R., Allodi, G., Chiesa, A., Garlatti, E., Mitcov, D., Konstantatos, A., Pedersen, K. S., De Renzi, R., Piligkos, Stergios & Carretta, S., 2018, In: Journal of the American Chemical Society. 140, 31, p. 9814-9818 5 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Modular [Fe^III₈M^II₆]ⁿ⁺ (M^II = Pd, Co, Ni, Cu) Coordination Cages
Sanz, S., O'Connor, H. M., Comar, P., Baldansuren, A., Pitak, M. B., Coles, S. J., Weihe, Høgni, Chilton, N. F., McInnes, E. J. L., Lusby, P. J., Piligkos, Stergios & Brechin, E. K., 2018, In: Inorganic Chemistry. 57, 7, p. 3500-3506 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2017
Published
[M^III₂M^II₃]ⁿ⁺ trigonal bipyramidal cages based on diamagnetic and paramagnetic metalloligands
Sanz, S., O'Connor, H. M., Marti-Centelles, V., Comar, P., Pitak, M. B., Coles, S. J., Lorusso, G., Palacios, E., Evangelisti, M., Baldansuren, A., Chilton, N. F., Weihe, Høgni, McInnes, E. J. L., Lusby, P. J., Piligkos, Stergios & Brechin, E. K., 2017, In: Chemical Science. 8, p. 5526-5535 10 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2016
Published
A hexameric [Mn^III₁₈Na₆] wheel based on [Mn^III₃O]⁷⁺ sub-units
Manoli, M., Inglis, R., Piligkos, Stergios, Yanhua, L., Wernsdorfer, W., Brechin, E. K. & Tasiopoulos, A. J., 2016, In: Chemical Communications. 52, 87, p. 12829-12832 4 p.
Research output: Contribution to journal › Letter › Research › peer-review
Published
In-depth magnetic characterization of a [2 × 2] Mn(III) square grid using SQUID magnetometry, inelastic neutron scattering, and high-field electron paramagnetic resonance spectroscopy
Konstantatos, A., Bewley, R., Barra, A. L., Bendix, Jesper, Piligkos, Stergios & Weihe, Høgni, 2016, In: Inorganic Chemistry. 55, 20, p. 10377-10382 6 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Iridates from the molecular side
Pedersen, K. S., Bendix, Jesper, Tressaud, A., Durand, E., Weihe, Høgni, Salman, Z., Morsing, T. J., Woodruff, D. N., Lan, Y., Wernsdorfer, W., Mathonière, C., Piligkos, Stergios, Klokishner, S. I., Ostrovsky, S., Ollefs, K., Wilhelm, F., Rogalev, A. & Clérac, R., 2016, In: Nature Communications. 7, 7 p., 12195.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Solvothermal synthesis of discrete cages and extended networks comprising {Cr(III)₃O(O₂CR)₃(oxime)₃}^2- (R = H, CH₃, C(CH₃)₃, C₁₄H₉) building blocks
Houton, E., Comar, P., Pitak, M. B., Coles, S. J., Ryder, A. G., Piligkos, Stergios, Brechin, E. K. & Jones, L. F., 2016, In: RSC Advances. 6, 77, p. 73668-73676 9 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Spin crossover in Fe(II) complexes with N₄S₂ coordination
Arroyave, A., Lennartson, A., Dragulescu-Andrasi, A., Pedersen, K. S., Piligkos, Stergios, Stoian, S. A., Greer, S. M., Pak, C., Hietsoi, O., Hoa Phan, Hill, S., McKenzie, C. J. & Shatruk, M., 2016, In: Inorganic Chemistry. 55, 12, p. 5904-5913 10 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Structurally flexible and solution stable [Ln₄TM₈(OH)₈(L)₈(O₂CR)₈(MeOH)_y](ClO₄)₄: a playground for magnetic refrigeration
Hooper, T. N., Inglis, R., Lorusso, G., Ujma, J., Barran, P. E., Uhrin, D., Schnack, J., Piligkos, Stergios, Evangelisti, M. & Brechin, E. K., 2016, In: Inorganic Chemistry. 55, 20, p. 10535-10546 12 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Toward molecular 4f single-ion magnet qubits
Pedersen, K. S., Ariciu, A., McAdams, S., Weihe, Høgni, Bendix, Jesper, Tuna, F. & Piligkos, Stergios, 2016, In: Journal of the American Chemical Society. 138, 18, p. 5801-5804 4 p.
Research output: Contribution to journal › Letter › Research › peer-review
Published
[Cr^III₈M^II₆]ⁿ⁺ (M^II = Cu, Co) face-centred, metallosupramolecular cubes
O'Connor, H. M., Sanz, S., Pitak, M. B., Coles, S. J., Nichol, G. S., Piligkos, Stergios, Lusby, P. J. & Brechin, E. K., 2016, In: CrystEngComm. 18, 26, p. 4914-4920 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2015
Published
Crystal structure of trihydrogen bis{[1,1,1-tris(2-oxidoethylaminomethyl)ethane]cobalt(III)} trinitrate
Sethi, W., Johannesen, H. V., Morsing, T. J., Piligkos, Stergios & Weihe, Høgni, 2015, In: Acta Crystallographica Section E. 71, 12, p. m275-m276, sup1-sup5 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Design of single-molecule magnets: insufficiency of the anisotropy barrier as the sole criterion
Pedersen, K. S., Dreiser, J., Weihe, Høgni, Sibille, R., Johannesen, H. V., Sørensen, M. A., Nielsen, B. E., Sigrist, M., Mutka, H., Rols, S., Bendix, Jesper & Piligkos, Stergios, 2015, In: Inorganic Chemistry. 54, 15, p. 7600-7606 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Facile interchange of 3d and 4f ions in single-molecule magnets: stepwise assembly of [Mn₄], [Mn₃Ln] and [Mn₂Ln₂] cages within Calix[4]arene scaffolds
Palacios, M. A., McLellan, R., Beavers, C. M., Teat, S. J., Weihe, Høgni, Piligkos, Stergios, Dalgarno, S. J. & Brechin, E. K., 2015, In: Chemistry: A European Journal. 21, 31, p. 11212-11218 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Linked supramolecular building blocks for enhanced cluster formation
McLellan, R., Palacios, M. A., Beavers, C. M., Teat, S. J., Piligkos, Stergios, Brechin, E. K. & Dalgarno, S. J., 2015, In: Chemistry: A European Journal. 21, 7, p. 2804-2812 9 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Magnetic and magnetocaloric properties of an unusual family of carbonate-panelled [Ln^III₆Zn^II₂] cages
Sethi, W., Sanz, S., Pedersen, K. S., Sørensen, M. A., Nichol, G. S., Lorusso, G., Evangelisti, M., Brechin, E. K. & Piligkos, Stergios, 2015, In: Dalton Transactions (Print Edition). 44, 22, p. 10315-10320 6 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Reversible guest binding in a non-porous Fe^II coordination polymer host toggles spin crossover
Lennartson, A., Southon, P., Sciortino, N. F., Kepert, C. J., Frandsen, C., Mørup, S., Piligkos, Stergios & McKenzie, C. J., 2015, In: Chemistry: A European Journal. 21, 45, p. 16066-16072 7 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
[Cr^III₈M^II₆]¹²⁺ Coordination Cubes (M^II=Cu, Co)
Sanz, S., O'Connor, H. M., Pineda, E. M., Pedersen, K. S., Nichol, G. S., Mønsted, O. V., Weihe, Høgni, Piligkos, Stergios, McInnes, E. J. L., Lusby, P. J. & Brechin, E. K., 2015, In: Angewandte Chemie International Edition. 54, 23, p. 6761-6764 4 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2014
Published
"Converting" an hexametallic Mn^III wheel to a dodecametallic Mn^III wheel via ligand oximation
Sanz, S., Frost, J. M., Pitak, M. B., Coles, S. J., Piligkos, Stergios, Lusby, P. J. & Brechin, E. K., 2014, In: Chemical Communications. 50, 25, p. 3310-3312 3 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Fluoride-bridged {Gd^III₃M^III₂} (M=Cr, Fe, Ga) molecular magnetic refrigerants
Pedersen, K. S., Lorusso, G., Morales, J. J., Weyhermüller, T., Piligkos, Stergios, Singh, S. K., Larsen, D., Schau-Magnussen, M., Rajaraman, G., Evangelisti, M. & Bendix, Jesper, 2014, In: Angewandte Chemie - International Edition. 53, 9, p. 2394-2397 4 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
[ReF₆]^2-: a robust module for the design of molecule-based magnetic materials
Pedersen, K. S., Sigrist, M., Sørensen, M. A., Barra, A. L., Weyhermuller, T., Piligkos, Stergios, Thuesen, C. A., Vinum, M. G., Mutka, H., Weihe, Høgni, Clerac, R. & Bendix, Jesper, 2014, In: Angewandte Chemie - International Edition. 53, 5, p. 1351-1354 4 p.
Research output: Contribution to journal › Journal article › Research › peer-review
2013
Published
Angular dependence of the exchange interaction in fluoride-bridged Gd^III-Cr^III complexes
Singh, S. K., Pedersen, K. S., Sigrist, M., Thuesen, C. A., Schau-Magnussen, M., Mutka, H., Piligkos, Stergios, Weihe, Høgni, Rajaraman, G. & Bendix, Jesper, 2013, In: Chemical Communications. 49, 49, p. 5583-5585 3 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
From antiferromagnetic to ferromagnetic exchange in a family of oxime-based Mn^III dimers: a magneto-structural study
Barros, W. P., Inglis, R., Nichol, G. S., Rajeshkumar, T., Rajaraman, G., Piligkos, Stergios, Stumpf, H. O. & Brechin, E. K., 2013, In: Dalton Transactions (Print Edition). 42, 47, p. 16510-16517 8 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Homo- and heterometallic planes, chains and cubanes
Meally, S. T., Taylor, S. M., Brechin, E. K., Piligkos, Stergios & Jones, L. F., 2013, In: Dalton Transactions (Print Edition). 42, 28, p. 10315-10325 11 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Homoleptic 5d fluoride complexes as modules for molecular spin-architectures
Pedersen, K. S., Clerac, R., Barra, A., Sibille, R., Probert, M., Meihaus, K., Dechambenoit, P., Sørensen, M. A., Sigrist, M., Weyhermüller, T., Weihe, Høgni, Piligkos, Stergios, Tressaud, A., Mutka, H., Bill, E., Long, J. R. & Bendix, Jesper, 2013. 1 p.
Research output: Contribution to conference › Poster › Research
Published
Jahn-Teller beads on a string: synthesis and magnetic properties of one-dimensional fluoride-bridged manganese(III)-systems
Sørensen, M. A., Pedersen, K. S., Piligkos, Stergios & Bendix, Jesper, 2013. 1 p.
Research output: Contribution to conference › Poster › Research
Published
Magnetic properties of fluoride-bridged linear chain S = 2 Heisenberg antiferromagnets
Sørensen, M. A., Pedersen, K. S., Piligkos, Stergios, Simeoni, G. & Bendix, Jesper, 2013.
Research output: Contribution to conference › Poster › Research
Published
New nanostructured materials: synthesis of dodecanuclear niII complexes and surface deposition studies
Pons-Balague, A., Piligkos, Stergios, Teat, S. J., Sanchez Costa, J., Shiddiq, M., Hill, S., Castro, G. R., Ferrer-Escorihuela, P. & Carolina Sanudo, E., 2013, In: Chemistry: A European Journal. 19, 27, p. 9064-9071 8 p.
Research output: Contribution to journal › Journal article › Research › peer-review
Published
Salicylaldoxime-supported nona- and tetrametallic Fe^IIIcages
Mason, K., Prescimone, A., Schau-Magnussen, M., Piligkos, Stergios, Tasker, P. A. & Brechin, E. K., 2013, In: Current Inorganic Chemistry. 3, 2, p. 76-85 10 p.
Research output: Contribution to journal › Journal article › Research › peer-review

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567 downloads
[Cr^III₈M^II₆]¹²⁺ Coordination Cubes (M^II=Cu, Co)
Research output: Contribution to journal › Journal article › Research › peer-review
Published
243 downloads
Chemical tunnel-splitting-engineering in a dysprosium-based molecular nanomagnet
Research output: Contribution to journal › Journal article › Research › peer-review
Published
157 downloads
Crystal structure of trihydrogen bis{[1,1,1-tris(2-oxidoethylaminomethyl)ethane]cobalt(III)} trinitrate
Research output: Contribution to journal › Journal article › Research › peer-review
Published